By J.P. Pradier and C.M. Pradier (Eds.)
This ebook derives from a workshop held in Sweden to ascertain the environmental implications of the dramatic elevate in carbon dioxide degrees within the surroundings within the final 50 years and to discover methods of mitigating greenhouse fuel emissions. This multi-disciplinary process makes it crucial examining not just for chemists yet for all engineers, biologists and environmentalists taken with this crucially very important factor
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Additional info for Carbon Dioxide Chemistry. Environmental Issues
X-ray diffraction structures of some Co complexes with C 0 indicated that the C 0 molecule is bent, suggesting that there is probably substantial electron donation to the C 0 ligand. Based on the electronic spectra of Co(en) (OH )C0 , which can be modeled as ligand-field transitions of Co" , a Co (C0 ") complex may actually be formed; less substantial electron donation may occur in other cases. Such an intermediate can then go on to react with protons to yield CO and OH' or HCOO" as illustrated in the catalytic cycle in Figure 1.
Ehrlich, S. Wohlrab, J. Wambach, H. -J. Freund, Vacuum. 1990, 42 10. 11. 12. 13. 14. 15. 16. 17. 18. 19. 20. 21. 22. 23. 24. 25. 26. 27. 28. 29. 30. 31. 32. 33. 34. 35. 36. 37. 38. 39. 40. 41. 42. 43. Carbon Dioxide Chemistry: Environmental Issues 41157; S. Wohlrab, D. Ehrlich, J. Wambach, H. -J. Freund, Surf. ScL 1989, 220. 243; J. Wambach, G. -J. Freund, H. Kuhlenbeck and M. Neumann. Surf. ScL 1989. 209. 159. F. Solymosi and A. Berko, J. CataL 1986. 101. 458. A Berko and F. Solymosi, Surf. ScL 1986, 171, L498.
One of the most effective catalysts in both phases is Rhodium. In a continuation of our research started more than 10 years ago in this field, in the present paper we give an account of our latest results obtained on the activation and catalytic reactions of C 0 over Rhodium. 2 1,2 2 1. ACTIVATION O F C 0 2 Activation of the rather inert and stable C 0 molecule on a metal catalyst is an important step in the conversion of C 0 into more valuable compounds ' . e. transformation of the stable linear structure into a more reactive bent form, is a key step in the activation of C 0 * .